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Using this sample and an ordinary Geiger counter, Libby and Anderson established the existence of naturally occurring carbon-14, matching the concentration predicted by Korff. Fortunately, Libby’s group developed an alternative. They surrounded the sample chamber with a system of Geiger counters that were calibrated to detect and eliminate the background radiation that exists throughout the environment.The assembly was called an “anti-coincidence counter.” When it was combined with a thick shield that further reduced background radiation and a novel method for reducing samples to pure carbon for testing, the system proved to be suitably sensitive.Known as radiocarbon dating, this method provides objective age estimates for carbon-based objects that originated from living organisms.The “radiocarbon revolution” made possible by Libby’s discovery greatly benefitted the fields of archaeology and geology by allowing practitioners to develop more precise historical chronologies across geography and cultures.Libby and graduate student Ernest Anderson (1920–2013) calculated the mixing of carbon across these different reservoirs, particularly in the oceans, which constitute the largest reservoir.Their results predicted the distribution of carbon-14 across features of the carbon cycle and gave Libby encouragement that radiocarbon dating would be successful.To test the technique, Libby’s group applied the anti-coincidence counter to samples whose ages were already known.

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We learned rather abruptly that these numbers, these ancient ages, are not known accurately; in fact, it is at about the time of the First Dynasty in Egypt that the first historical date of any real certainty has been established.” —Willard Libby, Nobel Lecture, 12 December 1960 The concept of radiocarbon dating focused on measuring the carbon content of discreet organic objects, but in order to prove the idea Libby would have to understand the earth’s carbon system.

Willard Libby (1908–1980), a professor of chemistry at the University of Chicago, began the research that led him to radiocarbon dating in 1945.

He was inspired by physicist Serge Korff (1906–1989) of New York University, who in 1939 discovered that neutrons were produced during the bombardment of the atmosphere by cosmic rays.

Radiocarbon dating would be most successful if two important factors were true: that the concentration of carbon-14 in the atmosphere had been constant for thousands of years, and that carbon-14 moved readily through the atmosphere, biosphere, oceans and other reservoirs—in a process known as the carbon cycle.

In the absence of any historical data concerning the intensity of cosmic radiation, Libby simply assumed that it had been constant.

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